ICEM’05: The 10th International Conference on Environmental Remediation and Radioactive Waste Management September 4-8, 2005, Scottish Exhibition & Conference Centre, Glasgow, Scotland |
S. Croft and W. Russ
Canberra Industries, Inc.
Abstract
The non destructive assay of special nuclear materials in storage
containers or as waste items often calls for the full energy peak efficiency
to be estimated in geometries which may be adequately described by the far
field approximation. The principle energy range of interest for materials
such as Pu + 241Am and HEU is below 500 keV. Small volume LEGe detectors
were once required for such applications where high resolution was needed to
extract information from the complex spectral regions. Recently, large volume
planar detectors called Broad Energy Ge (BEGe) detectors have become available.
BEGe detectors offer high resolution at low energy, as with LEGe detectors,
but with higher efficiency based on greater solid angle and thickness. However,
significantly changing detector dimensions requires an examination of the
adequacy of functions used to estimate and trend efficiencies. In this work
we discuss how the full energy peak efficiency of such planar detectors may
be estimated simply from the crystal and encapsulation dimensions. A new semi-empirical
formula is presented for the calculation and parameterization of the characteristic
far field full energy peak efficiency for energies below the pair production
threshold. The formula is an extension of the any interaction model with
allowance for the escape of fluorescent x-rays and secondary scattered radiation.
A database of sixteen such planar detectors with a wide variety of dimensions,
covering volumes from ~8 to ~150 cm3, is used to validate and verify
the method. In principal, this simple and quick to apply method is absolute
given accurate dimensions of the active volume, thickness of any frontal dead
layer and details of the end cap. Alternatively it can be used as a fitting
function to interpolate or extrapolate experimental data. The results show
that under the conditions examined, the formula is capable of reproducing measured
efficiencies to within a few percent over the energy range of interest.
Introduction
The non destructive assay of SNM in storage containers or as waste items often
calls for the full energy peak (FEP) efficiency to be estimated in geometries
which may be adequately described by the far field approximation (source to
detector separation much larger than detector dimensions) and sources primarily
in front of the detector. The principle energy range of interest for materials
such as Pu + 241Am and highly enriched uranium (HEU) is below 500 keV. This
range also covers the primary range for low energy mode relative isotopic measurements
of Pu by multi-group analysis methods. Small volume LEGe detectors were once
popular for such applications where high resolution was needed to extract information
from the complex spectral regions. Recently large volume planar detectors,
so called Broad Energy Ge or BEGe detectors, have become available. These offer
high energy resolution at low energies as before but with higher efficiency
because of solid angle and thickness.
In this work it is discussed how the FEP efficiency, ξ FEP, of such planar
detectors may be estimated simply from the crystal dimensions and those of
its encapsulation. The approach may be used to estimate the absolute efficiency
from fabrication information, as a means to fit absolute experimental data
or to fit relative efficiency profiles as would be called for in relative isotopics
analysis codes.